Spin-isospin Model of Nav 2 O 5

نویسنده

  • M. V. Mostovoy
چکیده

We argue that in the quarter-filled ladder compound NaV2O5 the quasione-dimensional spin system is strongly coupled to a low-energy antiferroelectric mode of the excitonic type. This mode results from the interplay between the electron hopping along the rungs of the vanadium two-leg ladders and the Coulomb repulsion between electrons. The charge ordering observed in sodium vanadate at Tc = 34K corresponds to the softening of the antiferroelectric mode. We consider the spin-isospin model, which describes the spin and low-energy charge degrees of freedom in sodium vanadate. Within this model we explain the observed anomalous temperature-dependence of the dielectric susceptibility at Tc and the midinfrared absorption continuum. We identify the broad structure in the low-energy optical absorption spectrum of NaV2O5 with the continuum formed by two spinons and one low-energy charge excitation. Spin-isospin model of NaV2O5 M. V. Mostovoy, J. Knoester, and D. I. Khomskii Theoretical Physics Institute and Materials Science Center, University of Groningen, Nijenborgh 4, 9747 AG Groningen, The Netherlands

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تاریخ انتشار 2008